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, the intrinsic partial molar volume) (c) limiting [] measured using viscometry and HPSEC-MALS in the 0.1-0.5M (LiNO 3 ) range, then extrapolated to charge neutralization and corrected taking into account gum polydispersity, (d) R H was calculated from measures of [] then extrapolated at charge neutralization and corrected according to the polydispersity. Values into parentheses correspond to R H obtained in 0.1 M LiNO 3 using DOSY-NMR, (e) R G was obtained from HPSEC-MALS measurements using only molecules with R G higher than 10 nm. (f) Experimental viscosity increment () was obtained from = ( ) [] v ° or estimated, (g) Hydration numbers calculated from hydrostatic volumetric properties of HIC-F1, HIC-F2 and HIC-F3 or estimated, s °, s ° and E° were calculated from measurements of density and sound velocity, (b) calculated from (1-M )*100, where M is the packing density (= V vdW /V M where V dvW is the van der Waals partial molar volume and V M is

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, Biomacromolecules, vol.17, pp.1198-1204, 2016.

G. O. Philips, S. Takigami, and M. Takigami, Hydration characteristics of the gum exudate from acacia senegal, Food Hydrocolloids, vol.10, pp.11-19, 1996.

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P. A. Williams and G. O. Philips, Gum arabic, Handbook of hydrocolloids, pp.155-168, 2000.

D. Renard, L. Lavenant-gourgeon, M. C. Ralet, and C. Sanchez, Acacia senegal gum: Continuum of molecular species differing by their protein to sugar ratio; molecular weight and charges, Biomacromolecules, pp.2637-2649, 2006.

O. H. Idris, P. A. Williams, and G. O. Phillips, Gum arabic's journey from tree to end user, 2012.
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D. Verbeken and D. Dierckx-s.;-k, Exudate gums: Occurence, production, and applications, Applied Microbiology Biotechnology, vol.63, pp.10-21, 2003.
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A. M. Islam, G. O. Phillips, A. Sljivo, M. J. Snowden, and P. A. Williams, A review of recent developments on the regulatory, structural and functional aspects of gum arabic, Food Hydrocolloids, vol.11, pp.493-505, 1997.

D. M. Anderson, M. M. Bridgeman, J. G. Farquhar, and C. G. Mcnab, The chemical characterization of the test article used in toxicological studies of gum arabic (acacia senegal (l.) willd), International Tree Crops Journal, vol.2, pp.245-254, 1983.

R. C. Randall, G. O. Phillips, and P. A. Williams, Fractionation and characterization of gum from acacia senegal, Food Hydrocolloids, vol.3, pp.65-75, 1989.
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C. Flindt, S. Alassaf, G. Phillips, and P. Williams, Studies on acacia exudate gums. Part v. Structural features of acacia seyal, Food Hydrocolloids, vol.19, pp.687-701, 2005.

L. Lopez-torrez, M. Nigen, P. Williams, T. Doco, and C. Sanchez, Acacia senegal vs. Acacia seyal gums-part 1: Composition and structure of hyperbranched plant exudates, Food Hydrocolloids, vol.51, pp.41-53, 2015.

D. M. Anderson and J. F. Stoddart, Studies on uronic acid materials. Part xv. The use of molecular-sieve chromatography on acacia senegal gum (gum arabic), Carbohydrate Research, vol.2, pp.104-114, 1966.
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A. E. Clarke, R. L. Anderson, and B. A. Stone, Form and function of arabinogalactans and arabinogalactan-proteins, Phytochemistry, vol.18, pp.521-540, 1979.

P. A. Williams, G. O. Philips, and R. C. Randall, Structure-function relantionships of gum arabic

, Gums and stabilizers for the industry 5, pp.25-36, 1990.

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D. M. Anderson, The amino acid composition and quantitative sugaramino acid relationships in sequential smithdegradation products from acacia polyacantha gum. Food Additives & Contaminants, vol.3, pp.123-132, 1986.

O. H. Idris, P. A. Williams, and G. O. Phillips, Characterisation of gum from acacia senegal trees of different age and location using multidetection gel permation chromatography

, Food Hydrocolloids, pp.379-388, 1998.

S. Assaf, G. Phillips, and P. Williams, Studies on acacia exudate gums. Part i: The molecular weight of gum exudate, Food Hydrocolloids, vol.19, pp.647-660, 2005.

K. A. Karamalla, N. E. Siddig, and M. E. Osman, Analytical data for acacia senegal var, Senegal gum samples collected between, 1993.

, Annexes 199 from sudan, Food Hydrocolloids, vol.12, pp.373-378, 1998.

T. Mahendran, P. Williams, G. Phillips, S. Alassaf, and T. Baldwin, New insights into the structural characteristics of the arabinogalactanprotein (agp) fraction of gum arabic, Journal of Agricultural and Food Chemistry, pp.9269-9276, 2008.

C. Sanchez, C. Schmitt, E. Kolodziejczyk, A. Lapp, C. Gaillard et al., The acacia gum arabinogalactan fraction is a thin oblate ellipsoid: A new model based on small-angle neutron scattering and ab initio calculation

, Biophysical Journal, vol.94, pp.629-639, 2008.

D. Renard, L. Lavenant-gourgeon, A. Lapp, M. Nigen, and C. Sanchez, Enzymatic hydrolysis studies of arabinogalactan-protein structure from acacia gum: The self-similarity hypothesis of assembly from a common builiding block

, Carbohydrate Polymers, vol.112, pp.648-661, 2014.

D. Renard, E. Lepvrier, C. Garnier, P. Roblin, M. Nigen et al., Structure of glycoproteins from acacia gum: An assembly of ring-like glycoproteins modules, Carbohydrate Polymers, vol.99, pp.736-747, 2014.
URL : https://hal.archives-ouvertes.fr/hal-01064003

S. Al-assaf, G. O. Phillips, H. Aoki, and Y. Sasaki, Characterization and properties of acacia senegal (l.) willd. Var. Senegal with enhanced properties (acacia (sen) super gum? ): Part 1-controlled maturation of acacia senegal var. Senegal to increase viscoelasticity, Food Hydrocolloids, vol.21, pp.319-328, 2007.

S. Al-assaf, G. Phillips, and P. Williams, Studies on acacia exudate gums: Part ii. Molecular weight comparison of the vulgares and gummiferae series of acacia gums, Food Hydrocolloids, vol.19, pp.661-667, 2005.

S. Al-assaf, M. Sakata, C. Mckenna, H. Aoki, and G. O. Phillips, Molecular associations in acacia gums, Structural Chemistry, vol.20, pp.325-336, 2009.

O. Castellani, S. Al-assaf, M. Axelos, G. O. Phillips, and M. Anton, Hydrocolloids with emulsifying capacity. Part 2-adsorption properties at the nhexadecane-water interface, Food Hydrocolloids, vol.24, pp.121-130, 2010.
URL : https://hal.archives-ouvertes.fr/hal-00662924

M. Elmanan, S. Al-assaf, G. O. Phillips, and P. A. Williams, Studies on acacia exudate gums: Part vi. Interfacial rheology of acacia senegal and acacia seyal, Food Hydrocolloids, vol.22, pp.682-689, 2008.

D. Renard, C. Garnier, A. Lapp, C. Schmitt, and C. Sanchez, Structure of arabinogalactan-protein from acacia gum: From porous ellipsoids to supramolecular architectures, Carbohydrate Polymers, vol.90, pp.322-332, 2012.
URL : https://hal.archives-ouvertes.fr/inserm-00870990

V. Mejia-tamayo, M. Nigen, R. Apolinar-valiente, T. Doco, P. Williams et al., Flexibility and hydration of amphiphilic hyperbranched arabinogalactan-protein from plant exudate: A volumetric perspective, Colloids and Interfaces, vol.2, p.11, 2018.
URL : https://hal.archives-ouvertes.fr/hal-02154396