M. Zéphoris, Pluies acides en France, Poll. Atm, vol.103, pp.159-165, 1984.

V. Ramaswamy, Radiative forcing of climate change. In Climate Change: The Scientific Basis. (Cambridge, pp.346-416, 2001.

N. Bellouin, Estimation de l'effet direct des aérosols à partir de la modélisation et de la télédétection passive, 2003.

M. Z. Jacobson, Strong radiative heating due to the mixing state of black carbon in atmospheric aerosols, Nature, vol.409, issue.6821, pp.695-697, 2001.
DOI : 10.1038/35055518

K. R. Spurny, On the physics, chemistry and toxicology of ultrafine anthropogenic, atmospheric aerosols (UAAA): new advances, Toxicology Letters, vol.96, issue.1-2, pp.96-97, 1998.
DOI : 10.1016/S0378-4274(98)00080-0

J. M. Haywood, P. N. Francis, M. D. Glew, T. , and J. P. , Optical properties and direct radiative effect of Saharan dust: A case study of two Saharan dust outbreaks using aircraft data, Journal of Geophysical Research: Atmospheres, vol.2, issue.3, pp.18417-18430, 2001.
DOI : 10.1029/2000JD900319

P. K. Quinn, D. J. Coman, V. N. Kapustin, T. S. Bates, and D. S. Covert, Aerosol optical properties in the marine boundary layer during the First Aerosol Characterization Experiment (ACE 1) and the underlying chemical and physical aerosol properties, Journal of Geophysical Research: Atmospheres, vol.17, issue.D13, pp.16547-16563, 1998.
DOI : 10.1029/97JD02345

I. N. Sokolik, D. M. Winker, G. Bergametti, D. A. Gillette, G. Carmichael et al., Introduction to special section: Outstanding problems in quantifying the radiative impacts of mineral dust, Journal of Geophysical Research: Atmospheres, vol.106, issue.D16, 2001.
DOI : 10.1029/2000JD900498

S. Lafon, J. Rajot, S. Alfaro, and A. Gaudichet, Quantification of iron oxides in desert aerosol, Atmospheric Environment, vol.38, issue.8, pp.1211-1218, 2004.
DOI : 10.1016/j.atmosenv.2003.11.006

I. Chiapello, G. Bergametti, B. Chatenet, P. Bousquet, F. Dulac et al., Origins of African dust transported over the northeastern tropical Atlantic, Journal of Geophysical Research: Atmospheres, vol.45, issue.D12, 1997.
DOI : 10.1029/97JD00259

D. Tanré, J. Haywood, J. Pelon, J. F. Léon, B. Chatenet et al., Measurement and modelling of the Saharan dust radiative impact: Overview of the Saharan Dust Experiment (SHADE) J, 2003.

J. Wang, P. , G. Li, X. Zhu, J. Reinert et al., Source identification of lead pollution in the Bibliographie atmosphere of Shanghai city by analyzing single aerosol particles (SAP), Environ. Sci, 2000.

F. Adams, Synchrotron radiation micro-X-ray fluorescence analysis: A tool to increase accuracy in microscopic analysis, Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, vol.199, pp.375-381, 2003.
DOI : 10.1016/S0168-583X(02)01563-X

J. N. Smith, K. F. Moore, P. H. Mcmurry, and F. L. Eisele, Atmospheric Measurements of Sub-20 nm Diameter Particle Chemical Composition by Thermal Desorption Chemical Ionization Mass Spectrometry, Aerosol Science and Technology, vol.34, issue.2, pp.100-110, 2004.
DOI : 10.1080/02786820252883856

S. Sobanska, N. Ricq, A. Laboudigue, R. Guillermo, C. Brémard et al., Microchemical Investigations of Dust Emitted by a Lead Smelter, Environmental Science & Technology, vol.33, issue.9, pp.1334-1339, 1999.
DOI : 10.1021/es9805270

Y. Batonneau, J. Laureyns, J. Merlin, and C. Brémard, Self-modeling mixture analysis of Raman microspectrometric investigations of dust emitted by lead and zinc smelters, Analytica Chimica Acta, vol.446, issue.1-2, pp.23-37, 2001.
DOI : 10.1016/S0003-2670(01)00909-6
URL : https://hal.archives-ouvertes.fr/hal-00279677

Y. Batonneau, C. Brémard, L. Gengembre, J. Laureyns, L. Maguer et al., Sources of Airborne Nonferrous Metals within the 3-km Zone of Lead/Zinc Smelters, Environmental Science & Technology, vol.38, issue.20, pp.5281-5289, 2004.
DOI : 10.1021/es0497173
URL : https://hal.archives-ouvertes.fr/hal-00269860

Y. Batonneau, C. Brémard, J. Laureyns, M. , and J. , Microscopic and imaging Raman scattering study of PbS and its photo-oxidation products, Journal of Raman Spectroscopy, vol.32, issue.411, pp.1113-1119, 2000.
DOI : 10.1002/1097-4555(200012)31:12<1113::AID-JRS653>3.0.CO;2-E

S. Caquineau, A. Gaudichet, L. Gomes, L. , and M. , Mineralogy of Saharan dust transported over northwestern tropical Atlantic Ocean in relation to source regions, Journal of Geophysical Research, vol.45, issue.3???4, p.4251, 2002.
DOI : 10.1029/2000JD000247

E. Drab, A. Gaudichet, J. Jaffrezo, C. , and J. , Mineral particles content in recent snow at Summit (Greenland), Atmospheric Environment, vol.36, issue.34, pp.5365-3676, 2002.
DOI : 10.1016/S1352-2310(02)00470-3

C. L. Gregory, H. A. Nullens, R. H. Gijbels, P. J. Van-espen, I. Geuens et al., Automated Particle Analysis of Populations of Silver Halide Microcrystals by Electron Probe Microanalysis under Cryogenic Conditions, Analytical Chemistry, vol.70, issue.13, pp.2551-2559, 1998.
DOI : 10.1021/ac9710644

A. Laskin and J. P. And-cowin, Automated Single-Particle SEM/EDX Analysis of Submicrometer Particles down to 0.1 ??m, Analytical Chemistry, vol.73, issue.5, pp.1023-1029, 2001.
DOI : 10.1021/ac0009604

Y. Mamane, R. Willis, and T. Conner, Evaluation of Computer-Controlled Scanning Electron Microscopy Applied to an Ambient Urban Aerosol Sample, Aerosol Science and Technology, vol.34, issue.1, 2001.
DOI : 10.1080/02786820118842

F. Adams, Sampling and analysis of aerosols, Pure and Applied Chemistry, vol.55, issue.12, pp.1925-1942, 1983.
DOI : 10.1351/pac198355121925

W. Jambers, D. Bock, L. Van-grieken, and R. , Recent advances in the analysis of individual environmental particles. A review, The Analyst, vol.120, issue.3, pp.681-692, 1995.
DOI : 10.1039/an9952000681

D. Bock, L. A. Van-grieken, and R. E. , Single particle analysis techniques, Analytical Chemistry of Aerosols, pp.243-275, 1999.

C. Ro, S. Hoornaert, and R. Van-grieken, Assessment of homogeneity of candidate reference material at the nanogram level and investigation on representativeness of single particle analysis using electron probe X-ray microanalysis, Analytica Chimica Acta, vol.389, issue.1-3, 1999.
DOI : 10.1016/S0003-2670(99)00160-9

J. Watt, Automated feature analysis in the scanning electron microscope. Microsc. Anal, pp.25-28, 1990.

J. J. Mulders and R. J. Endert, The influence of parameter settings on speed and accuracy of automatic particle analysis, Micron and Microscopica Acta, vol.23, issue.1-2, pp.205-206, 1992.
DOI : 10.1016/0739-6260(92)90140-9

R. W. Linton, M. E. Farmer, P. K. Hopke, and D. F. Natusch, Determination of the sources of toxic elements in environmental particles using microscopic and statistical analysis techniques, Environment International, vol.4, issue.5-6, pp.453-461, 1980.
DOI : 10.1016/0160-4120(80)90026-4

P. C. Bernard and R. E. Van-grieken, Classification of estuarine particles using automated electron microprobe analysis and multivariate techniques, Environmental Science & Technology, vol.20, issue.5, 1986.
DOI : 10.1021/es00147a005

D. A. Saucy, J. A. Anderson, and P. R. Buseck, Cluster analysis applied to atmospheric aerosol samples from the Norwegian Arctic, Atmospheric Environment (1967), vol.21, issue.7, pp.1649-1657, 1987.
DOI : 10.1016/0004-6981(87)90326-X

C. Xhoffer, P. Bernard, R. Van-grieken, and L. Van-der-auwera, Chemical characterization and source apportionment of individual aerosol particles over the North Sea and the English Channel using multivariate techniques, Environmental Science & Technology, vol.25, issue.8, pp.1470-1478, 1991.
DOI : 10.1021/es00020a017

B. Treiger, I. Bondarenko, H. Van-malderen, and R. Van-grieken, Elucidating the composition of atmospheric aerosols through the combined hierarchical, nonhierarchical and fuzzy clustering of large electron probe microanalysis data sets, 1995.

D. Bock, L. A. Treiger, B. Van-der-auwera, L. Van-grieken, and R. , Extraction of environmental information from large aerosol data sets through combined application of cluster and factor analyses, Microchimica Acta, vol.25, issue.3-4, pp.191-200, 1998.
DOI : 10.1007/BF01243049

J. Osán, J. De-hoog, A. Worobiec, C. Ro, K. Oh et al., Application of chemometric methods for classification of atmospheric particles based on thin-window electron probe microanalysis data, Analytica Chimica Acta, vol.446, issue.1-2, pp.211-222, 2001.
DOI : 10.1016/S0003-2670(01)00935-7

C. Ro, K. Oh, H. Kim, Y. P. Kim, C. B. Lee et al., Electron Probe X-ray Microanalysis:?? A Direct Proof of Nitrate Formation from Sea Salts, Environmental Science & Technology, vol.35, issue.22, pp.4487-4494, 2001.
DOI : 10.1021/es0155231

A. Laskin, M. J. Iedema, and J. P. And-cowin, Time-Resolved Aerosol Collector for CCSEM/EDX Single-Particle Analysis, Aerosol Science and Technology, vol.40, issue.3, pp.246-260, 2003.
DOI : 10.1021/es990567j

D. Bock, L. A. Van-malderen, H. Van-grieken, and R. , Individual Aerosol Particle Composition Variations in Air Masses Crossing the North Sea, Environmental Science & Technology, vol.28, issue.8, pp.1513-1520, 1994.
DOI : 10.1021/es00057a021

J. De-hoog, J. Osán, I. Szalóki, K. Eyckmans, A. Worobiec et al., Thin-window electron probe X-ray microanalysis of individual atmospheric particles above the North Sea, Atmospheric Environment, vol.39, issue.18, pp.3231-3242, 2005.
DOI : 10.1016/j.atmosenv.2005.02.025

J. A. Anderson, P. R. Buseck, and T. L. Patterson, Characterization of the Bermuda troposheric aerosol by combined individual-particle and bulk-aerosol analysis, 1996.

W. Jambers, D. Bock, L. Van-grieken, and R. , Applications of micro-analysis to individual environmental particles, Fresenius' Journal of Analytical Chemistry, vol.355, issue.5-6, pp.521-527, 1996.
DOI : 10.1007/s0021663550521

S. Hoornaert, R. H. Godoi, and R. Van-grieken, Elemental and Single Particle Aerosol Characterisation at a Background Station in Kazakhstan, Journal of Atmospheric Chemistry, vol.48, issue.3, pp.301-315, 2004.
DOI : 10.1023/B:JOCH.0000044432.74476.b0

Y. Gao, A. , and J. R. , Characteristics of Chinese aerosols determined by individual-particle analysis, Journal of Geophysical Research: Atmospheres, vol.22, issue.D16, pp.18037-18045, 2001.
DOI : 10.1029/2000JD900725

Y. Iwasaka, G. Y. Shi, M. Yamada, A. Matsuki, D. Trochkine et al., Importance of dust particles in the free troposphere over the Taklamakan Desert: Electron microscopic experiments of particles collected with a balloonborne particle impactor at Dunhuang, China, Journal of Geophysical Research, vol.40, issue.D23, p.8644, 2003.
DOI : 10.1029/2002JD003270

S. Sobanska, C. Coeur, W. Maenhaut, A. , and F. , SEM-EDX characterisation of tropospheric aerosols in the Negev desert (Israel), Journal of Atmospheric Chemistry, vol.44, issue.3, pp.299-322, 2003.
DOI : 10.1023/A:1022969302107

C. Ro, H. Hwang, H. Kim, Y. Chun, and R. Van-grieken, Particle Electron Probe X-ray Microanalysis, Environmental Science & Technology, vol.39, issue.6, pp.1409-1419, 2005.
DOI : 10.1021/es049772b

K. Okada, Y. Qinb, K. , and K. , Elemental composition and mixing properties of atmospheric mineral particles collected in Hohhot, China, Atmospheric Research, vol.73, issue.1-2, pp.45-67, 2005.
DOI : 10.1016/j.atmosres.2004.08.001

B. Sitzmann, M. Kendall, J. Watt, W. , and I. , Characterisation of airborne particles in London by computer-controlled scanning electron microscopy, Science of The Total Environment, vol.241, issue.1-3, 1999.
DOI : 10.1016/S0048-9697(99)00326-5

K. A. Katrinak, J. R. Anderson, and P. R. Buseck, Individual Particle Types in the Aerosol of Phoenix, Arizona, Environmental Science & Technology, vol.29, issue.2, pp.321-329, 1995.
DOI : 10.1021/es00002a007

A. Piña, A. Torres-villaseñor, G. , M. Fernández, M. et al., Scanning electron microscope and statistical analysis of suspended heavy metal particles in San Luis Potosi, Mexico, Atmospheric Environment, vol.34, issue.24, pp.4103-4112, 2000.
DOI : 10.1016/S1352-2310(99)00526-9

T. L. Conner, G. A. Norris, M. S. Landis, W. , and R. W. , Individual particle analysis of indoor, outdoor, and community samples from the 1998 Baltimore particulate matter study, Atmospheric Environment, vol.35, issue.23, pp.3935-3946, 2001.
DOI : 10.1016/S1352-2310(01)00191-1

R. Maura-de-miranda, M. De-fátima-andrade, A. Worobiec, and R. Van-grieken, Characterisation of aerosol particles in the S??o Paulo Metropolitan Area, Atmospheric Environment, vol.36, issue.2, 2002.
DOI : 10.1016/S1352-2310(01)00363-6

C. Ro, H. Kim, K. Oh, S. K. Yea, C. B. Lee et al., Electron Probe X-ray Microanalysis, Environmental Science & Technology, vol.36, issue.22, pp.4770-4776, 2002.
DOI : 10.1021/es025697y
URL : https://hal.archives-ouvertes.fr/hal-00712636

R. Van-grieken, K. Gysels, S. Hoornaert, P. Joos, J. Osán et al., Characterisation of individual aerosol particles for atmospheric and cultural heritage studies. Water, Air and Soil Pollut, pp.215-228, 2000.

A. Chabas and R. A. Lefèvre, Chemistry and microscopy of atmospheric particulates at Delos (Cyclades???Greece), Atmospheric Environment, vol.34, issue.2, pp.225-238, 2000.
DOI : 10.1016/S1352-2310(99)00255-1

X. Liu, P. Van-espen, F. Adams, J. Cafmeyer, and W. Maenhaut, Biomass burning in Southern Africa: Individual particle characterization of atmospheric aerosols and savanna fire samples, Journal of Atmospheric Chemistry, vol.36, issue.2, pp.135-155, 2000.
DOI : 10.1023/A:1006387031927

M. Ebert, J. Dahmen, P. Hoffmann, and H. M. Ortner, Examination of clean room aerosol composition by total reflection X-ray analysis and electron probe microanalysis. Spectrochim, Acta B, vol.52, pp.967-975, 1997.

J. Injuk, J. Osán, R. Van-grieken, and K. Tsuji, Airborne Particles in the Miyagi Museum of Art in Sendai, Japan, Studied by Electron Probe X-ray Microanalysis and Energy Dispersive X-ray Fluorescence Analysis., Analytical Sciences, vol.18, issue.5, pp.561-566, 2002.
DOI : 10.2116/analsci.18.561

P. R. Buseck and M. Pósfai, Airborne minerals and related aerosol particles: Effects on climate and the environment, Natl. Acad. Sci. USA, pp.3372-3379, 1998.
DOI : 10.1073/pnas.96.7.3396

J. Kasparian, E. Frejafon, P. Rambaldi, J. Yu, B. Vezin et al., Characterization of urban aerosols using SEM-microscopy, X-ray analysis and Lidar measurements, Atmospheric Environment, vol.32, issue.17, pp.2957-2967, 1998.
DOI : 10.1016/S1352-2310(98)00013-2

C. Xhoffer, L. Wouters, and R. Van-grieken, Characterization of individual particles in the North Sea surface microlayer and underlying seawater: comparison with atmospheric particles, Environmental Science & Technology, vol.26, issue.11, pp.2151-2162, 1992.
DOI : 10.1021/es00035a013

W. Jambers, V. Dekov, and R. Van-grieken, Single particle characterisation of inorganic and organic North Sea suspension, Marine Chemistry, vol.67, issue.1-2, pp.17-32, 1999.
DOI : 10.1016/S0304-4203(99)00046-8

W. Jambers, V. Dekov, and R. Van-grieken, Single particle and inorganic characterization of rainwater collected above the North Sea, Science of The Total Environment, vol.256, issue.2-3, pp.133-150, 2000.
DOI : 10.1016/S0048-9697(00)00477-0

J. Osán, S. Kurunczi, S. Török, A. Worobiec, and R. Van-grieken, Application of Thin-Window EPMA to Environmental Problems in Hungary, Microchimica Acta, vol.139, issue.1-4, pp.111-117, 2002.
DOI : 10.1007/s006040200048

S. Hoornaert, Chemical characterisation of atmospheric aerosols: application in the context of air pollution and global climatic change, 2000.

D. L. Johnson, B. Mcintyre, R. Fortman, R. K. Stevens, H. et al., A chemical element comparison of individual particle analysis and bulk analysis methods, Scanning Electron Microsc, vol.1, pp.469-476, 1981.

M. S. Germani and P. R. Buseck, Automated scanning electron microscopy for atmospheric particle analysis, Analytical Chemistry, vol.63, issue.20, pp.2232-2237, 1991.
DOI : 10.1021/ac00020a008

P. Poelt, M. Schmied, I. Obernberger, T. Brunner, and J. Dahl, Automated analysis of submicron particles by computer-controlled scanning electron microscopy, Scanning, vol.28, issue.11, pp.92-100, 2002.
DOI : 10.1002/sca.4950240207

P. Van-espen, Quantitative microbeam analysis of particles, Microchimica Acta, vol.18, issue.1, pp.129-142, 1994.
DOI : 10.1007/BF01244537

A. Worobiec, A. Kaplinski, and R. Van-grieken, Ruthenium staining as an alternative preparation method for automated EPMA of individual biogenic and organic particles. X-Ray Spectrom, pp.245-252, 2005.

J. I. Goldstein, D. E. Newbury, P. Echlin, D. C. Joy, C. E. Lyman et al., Scanning Electron Microscopy and X-ray Microanalysis, J.R, 2003.

R. Bonetto, G. Castellano, and J. Trincavelli, Optimization of parameters in electron probe microanalysis. X-Ray Spectrom, pp.313-319, 2001.

B. Vekemans, K. Janssens, L. Vincze, F. Adams, and P. Van-espen, Analysis of X-ray spectra by iterative least squares (AXIL): new developments. X-ray Spectrom, pp.278-285, 1994.

R. A. Carlton, The effect of some instrument operating conditions on the x-ray microanalysis of particles in the environmental scanning electron microscope, Scanning, vol.179, issue.2, pp.85-91, 1997.
DOI : 10.1002/sca.4950190205

D. R. Lide, CRC Handbook of Chemistry and Physics, 1994.

P. Huang and B. Turpin, Reduction of sampling and analytical errors for electron microscopic analysis of atmospheric aerosols, Atmospheric Environment, vol.30, issue.24, pp.4137-4148, 1996.
DOI : 10.1016/1352-2310(96)00150-1

E. S. Windsor, D. E. Newbury, J. D. Kessler, C. , and P. H. , Boron substrate for particulate X-ray microanalysis, pp.920-921, 1999.

D. Mayer-worobiec and A. , Optimisation and application of different electron probe X-ray microanalysis approaches for the chemical characterisation of individual environmental particles, 2003.

C. Ro, K. Oh, H. Kim, Y. Chun, J. Osán et al., Chemical speciation of individual atmospheric particles using low-Z electron probe X-ray microanalysis:, Atmospheric Environment, vol.35, issue.29, pp.4995-5005, 2001.
DOI : 10.1016/S1352-2310(01)00287-4

J. A. Small, D. E. Newbury, A. , and J. T. , Electron-induced X-ray emission. In Handbook of X-ray Spectrometry, pp.811-931, 2002.

D. C. Joy, Monte Carlo Modeling for Electron Microscopy and Microanalysis, 1995.

R. A. Fletcher, J. A. Small, and J. H. Scott, Analysis of individual collected particles, Aerosol Measurement: Principles, Techniques, and Applications, pp.295-363, 2001.

V. D. Scott, G. Love, R. , and S. J. , Quantitative electron-probe microanalysis, 1995.

Z. Spolnik, J. Zhang, K. Wagatsuma, and K. Tsuji, Grazing-exit electron probe X-ray microanalysis of ultra-thin films and single particles with high-angle resolution, Analytica Chimica Acta, vol.455, issue.2, 2002.
DOI : 10.1016/S0003-2670(01)01601-4

J. A. Small, The analysis of particles at low accelerating voltages (<= 10 kV) with energy dispersive x-ray spectroscopy (EDS), Journal of Research of the National Institute of Standards and Technology, vol.107, issue.6, pp.555-566, 2002.
DOI : 10.6028/jres.107.047

C. Ro, J. Osán, and R. Van-grieken, Elements in Individual Environmental Particles Using Windowless EPMA, Analytical Chemistry, vol.71, issue.8, pp.1521-1528, 1999.
DOI : 10.1021/ac981070f

M. Schmied and P. Poelt, Particle Analysis by SEM/EDXS and Specimen Damage, Microchimica Acta, vol.139, issue.1-4, pp.171-177, 2002.
DOI : 10.1007/s006040200057

J. Osán, I. Szalóki, C. Ro, and R. Van-grieken, Light Element Analysis of Individual Microparticles Using Thin-Window EPMA, Microchimica Acta, vol.132, issue.2-4, pp.349-355, 2000.
DOI : 10.1007/s006040050079

J. Trincavelli and G. Castellano, MULTI: an interactive program for quantitation in EPMA. X-Ray Spectrom, pp.194-197, 1999.

B. Alfödy, J. Trincavelli, S. Török, and G. Castellano, Characterization of atmospheric particles by electron probe X-ray microanalysis, Scanning, vol.1, issue.6, pp.297-300, 2002.
DOI : 10.1002/sca.4950240603

J. T. Armstrong and P. R. Buseck, Quantitative chemical analysis of individual microparticles using the electron microprobe. Theoretical, Analytical Chemistry, vol.47, issue.13, pp.2178-2192, 1975.
DOI : 10.1021/ac60363a033

J. T. Armstrong and P. R. Buseck, A general characteristic fluorescence correction for the quantitative electron microbeam analysis of thick specimens, thin films and particles. X-Ray Spectrom, pp.172-182, 1985.

P. Hovington, D. Drouin, and R. Gauvin, CASINO: A new monte carlo code in C language for electron beam interaction -part I: Description of the program, Scanning, vol.4, issue.4, pp.1-14, 1997.
DOI : 10.1002/sca.4950190101

D. Drouin, P. Hovington, and R. Gauvin, CASINO: A new monte carlo code in C language for electron beam interactions-part II: Tabulated values of the mott cross section, Scanning, vol.40, issue.suppl. V, pp.20-28, 1997.
DOI : 10.1002/sca.4950190103

P. Hovington, D. Drouin, R. Gauvin, D. C. Joy, and N. Evans, CASINO: A new monte Carlo code in C language for electron beam interactions-part III: Stopping power at low energies, Scanning, vol.36, issue.1, pp.29-35, 1997.
DOI : 10.1002/sca.4950190104

I. Szalóki, J. Osán, C. Ro, and R. Van-grieken, Quantitative characterization of individual aerosol particles by thin-window electron probe microanalysis combined with iterative simulation. Spectrochim, Acta B, vol.55, pp.1017-1030, 2000.

Y. Li, X. Liu, S. Dong, P. Van-espen, A. et al., Investigation on the geometric and matrix effects and quantitative determination of K, Cl and S atomic fraction for biomass burning particles by Monte Carlo simulation, Analytica Chimica Acta, vol.459, issue.1, pp.93-106, 2002.
DOI : 10.1016/S0003-2670(02)00081-8

J. De-hoog, R. Godoi, A. Worobiec, and R. Van-grieken, Evaluation of electron probe X-ray microanalysis of single particles collected on TEM grids, EMAS 2003, 8th European Workshop on Modern Developments and Applications in Microbeam Analysis, 2003.

F. Bruynseels, H. Storms, and R. Van-grieken, Characterization of North Sea aerosols by individual particle analyses, Atmospheric Environment (1967), vol.22, issue.11, pp.2593-2602, 1988.
DOI : 10.1016/0004-6981(88)90493-3

A. Renoux and D. Boulaud, Les aérosols -Physique et métrologie, 1998.

P. Flament, Les métaux-traces associés aux aérosols atmosphériques : apports au milieu marin du littoral Nord-Pas de Calais, 1985.

P. Rolland, V. L. Carlino, and R. Vane, Improved Carbon Analysis with Evactron Plasma Cleaning, Microscopy and Microanalysis, 2004.
DOI : 10.1017/S1431927604880504

M. Prinz, G. Harlow, and J. Peters, Simon & Schuster's Guide to Rocks and Minerals, 1978.

A. Foucault, R. , and J. , Dictionnaire de géologie, 1995.

W. A. Deer, R. A. Howie, and J. Zussman, An Introduction to the Rock-Forming Minerals, 1992.

I. Bondarenko, B. Treiger, R. Van-grieken, and P. Van-espen, IDAS: a Windows based software package for cluster analysis, Spectrochimica Acta Part B: Atomic Spectroscopy, vol.51, issue.4, pp.441-456, 1996.
DOI : 10.1016/0584-8547(95)01448-9

J. M. Haywood and V. Ramaswamy, Global sensitivity studies of the direct radiative forcing due to anthropogenic sulfate and black carbon aerosols, Journal of Geophysical Research: Atmospheres, vol.15, issue.D6, 1998.
DOI : 10.1029/97JD03426

G. Myhre, F. Stordal, K. Restad, and I. S. Isaksen, Estimation of the direct radiative forcing due to sulfate and soot aerosols, Tellus B: Chemical and Physical Meteorology, vol.369, issue.5, pp.463-477, 1998.
DOI : 10.3402/tellusb.v50i5.16230

M. Z. Jacobson, A physically-based treatment of elemental carbon optics: Implications for global direct forcing of aerosols, Geophysical Research Letters, vol.28, issue.2, pp.217-220, 2000.
DOI : 10.1029/1999GL010968

M. Z. Jacobson and J. H. Seinfeld, Evolution of nanoparticle size and mixing state near the point of emission, Atmospheric Environment, vol.38, issue.13, pp.1839-1850, 2004.
DOI : 10.1016/j.atmosenv.2004.01.014

M. Choël, K. Deboudt, J. Osán, P. Flament, and R. , Elements in Single Atmospheric Particles on Boron Substrates by Automated Scanning Electron Microscopy???Energy-Dispersive X-ray Spectrometry, Analytical Chemistry, vol.77, issue.17, pp.5686-5692, 2005.
DOI : 10.1021/ac050739x

. Belgium, R. M. Harrison, and R. E. Van-grieken, Atmospheric Particles, 1998.

W. Jambers, L. De-bock, and R. Van-grieken, Applications of micro-analysis to individual environmental particles, Fresenius' Journal of Analytical Chemistry, vol.355, issue.5-6, pp.521-527, 1996.
DOI : 10.1007/s0021663550521

E. Frejafon, J. Kasparian, P. Rambaldi, J. Yu, B. Vezin et al., Three-dimensional analysis of urban aerosols by use of a combined lidar, scanning electron microscopy, and x-ray microanalysis, Applied Optics, vol.37, issue.12, pp.2231-2237, 1998.
DOI : 10.1364/AO.37.002231

B. Treiger, I. Bondarenko, H. Van-malderen, and R. Van-grieken, Elucidating the composition of atmospheric aerosols through the combined hierarchical, non-hierarchical and fuzzy clustering of large electron probe microanalysis data sets, Analytica Chimica Acta, vol.317, issue.1-3, pp.33-51, 1995.
DOI : 10.1016/0003-2670(95)00405-X

A. Laskin, M. J. Iedema, and J. P. Cowin, Quantitative Time-Resolved Monitoring of Nitrate Formation in Sea Salt Particles Using a CCSEM/EDX Single Particle Analysis, Environmental Science & Technology, vol.36, issue.23, pp.4948-4955, 2002.
DOI : 10.1021/es020551k

B. J. Krueger, V. H. Grassian, A. Laskin, J. P. Cowin, B. J. Krueger et al., The transformation of solid atmospheric particles into liquid droplets through heterogeneous chemistry: Laboratory insights into the processing of calcium containing mineral dust aerosol in the troposphere, Geophysical Research Letters, vol.106, issue.D9, pp.1148-1164, 2003.
DOI : 10.1029/2002GL016563

A. Laskin, D. J. Gaspar, W. Wang, S. W. Hunt, J. P. Cowin et al., Reactions at Interfaces As a Source of Sulfate Formation in Sea-Salt Particles, Science, vol.301, issue.5631, pp.340-344, 2003.
DOI : 10.1126/science.1085374

B. J. Krueger, V. H. Grassian, J. P. Cowin, and A. Laskin, Heterogeneous chemistry of individual mineral dust particles from different dust source regions: the importance of particle mineralogy, Atmospheric Environment, vol.38, issue.36, pp.6253-6261, 2004.
DOI : 10.1016/j.atmosenv.2004.07.010

M. Ebert, M. Inerle-hof, and S. Weinbruch, Environmental scanning electron microscopy as a new technique to determine the hygroscopic behaviour of individual aerosol particles, Atmospheric Environment, vol.36, issue.39-40, pp.5909-5916, 2002.
DOI : 10.1016/S1352-2310(02)00774-4

R. C. Hoffman, A. Laskin, and B. Finlayson-pitts, Sodium nitrate particles: physical and chemical properties during hydration and dehydration, and implications for aged sea salt aerosols, Journal of Aerosol Science, vol.35, issue.7, pp.869-887, 2004.
DOI : 10.1016/j.jaerosci.2004.02.003

C. Ro, K. Oh, J. Osán, J. De-hoog, A. Worobiec et al., Particles Using Ultrathin Window Electron Probe X-ray Microanalysis, Analytical Chemistry, vol.73, issue.19, pp.4574-4583, 2001.
DOI : 10.1021/ac010438x

I. Szaló-ki, C. Ro, J. Osán, and J. De-hoog, In X-ray Spectrometry: Recent Technological Advances, pp.569-592, 2004.

J. A. Small, D. E. Newbury, and J. Armstrong, In Handbook of X-ray Spectrometry, pp.811-931, 2002.

J. I. Goldstein, D. E. Newbury, P. Echlin, D. C. Joy, C. E. Lyman et al., Scanning Electron Microscopy and X-ray Microanalysis, Anal. Chem. Anal. Chem. Environ. Sci. Technol, vol.73, issue.28, pp.1023-1029, 1991.

B. Sitzmann, M. Kendall, and J. Watt, Characterisation of airborne particles in London by computer-controlled scanning electron microscopy, Science of The Total Environment, vol.241, issue.1-3, pp.63-73, 1999.
DOI : 10.1016/S0048-9697(99)00326-5

P. Huang, B. Turpin, R. A. Fletcher, J. A. Small, and J. H. Scott, Reduction of sampling and analytical errors for electron microscopic analysis of atmospheric aerosols, Aerosol Measurement: Principles, Techniques, and Applications, pp.4137-4148, 1996.
DOI : 10.1016/1352-2310(96)00150-1

C. Ro, J. Osán, I. Szaló-ki, J. De-hoog, and A. Worobiec, A Monte Carlo Program for Quantitative Electron-Induced X-ray Analysis of Individual Particles, Analytical Chemistry, vol.75, issue.4, pp.851-859, 2003.
DOI : 10.1021/ac025973r

B. Vekemans, K. Janssens, L. Vincze, and F. Adams, Van Espen, P. X-ray Spectrom, pp.278-285, 1994.

C. Ro, J. Osán, I. Szaló-ki, K. Oh, H. Kim et al., Determination of Chemical Species in Individual Aerosol Particles Using Ultrathin Window EPMA, Environmental Science & Technology, vol.34, issue.14, pp.3023-3030, 2000.
DOI : 10.1021/es9910661